01-09-2022 дата публикации
Номер: US20220277865A1
Reactor target assemblies are provided that can include a housing defining a perimeter of at least one volume and Np or Am spheres within the one volume. Reactor assemblies are provided that can include a reactor vessel and a bundle of target assemblies within the reactor vessel, at least one of the target assemblies comprising a housing defining a volume with Np or Am spheres being within the volume. Irradiation methods are also provided that can include irradiating Np or Am spheres within a nuclear reactor, then removing the irradiated spheres from the reactor and treating the irradiated spheres. 1. A method for producing spheres of Am , Np , or Pu , the method comprising:preparing a nitrate solution comprising Am, Np, or Pu;gelling the Am, Np, or Pu;providing the gelled Am, Np, or Pu through a conduit with another fluid to form gelled Am, Np, or Pu spheres; andwashing and drying gelled spheres to form solid Am, Np, or Pu spheres.2. The method of further comprising forming a mixed feed solution comprising the nitrate solution to gel the Am claim 1 , Np claim 1 , or Pu.3. The method of wherein the mixed feed solution comprises HMTA.4. The method of wherein the mixed feed solution comprises urea.5. The method of further comprising changing the temperature of the mixed feed solution to a point above freezing to gel the Am claim 2 , Np claim 2 , or Pu.6. The method of further comprising providing the gelled Am claim 1 , Np claim 1 , or Pu from the conduit to a forming fluid.7. The method of further comprising removing the forming fluid when washing the gelled spheres.8. The method of further comprising washing the gelled spheres with a solvent.9. The method of wherein the solvent is trichloroethylene and/or isopropyl alcohol.10. The method of wherein the solvent comprises ammonium hydroxide.11. The method of wherein the drying comprises heating the washed spheres.12. The method of wherein claim 11 , upon drying claim 11 , the spheres are rinsed with water and dried to ...
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